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GitHub will complain about any file committed over 50MB.
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The hard quota is 100MB. Everything larger has to go to LFS.
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LFS has a hard cap at 4GB for teams, but we are also metered.
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That is, using LFS has an inherent cost in terms of storage (how much you upload) and bandwidth (how much you download). In short, we should avoid using LFS. It solves nearly nothing.